Temporal dynamics of femtosecond-TALIF of atomic hydrogen and oxygen in a nanosecond repetitively pulsed discharge-assisted methane–air flame

نویسندگان

چکیده

Abstract The temporal dynamics of the spatial distribution atomic hydrogen and oxygen in a lean methane–air flame, forced by nanosecond repetitively pulsed discharge-induced plasma, are investigated via femtosecond two-photon absorption laser-induced fluorescence technique. Plasma luminescence that interferes with from H O atoms was observed to decay completely within 15 ns, which is minimum delay required for imaging measurements respect discharge occurrence. During discharge, excited state rather than ground state, produced electron-impact dissociation processes, detected at flame front. It found evolution intensity during cycle 100 µ s between two pulses remains constant. Finally, time O-atoms fresh mixture about 2 s, suggests faster reaction methane air.

برای دانلود باید عضویت طلایی داشته باشید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Species and temperature measurements of methane oxidation in a nanosecond repetitively pulsed discharge.

Speciation and temperature measurements of methane oxidation during a nanosecond repetitively pulsed discharge in a low-temperature flow reactor have been performed. Measurements of temperature and formaldehyde during a burst of pulses were made on a time-dependent basis using tunable diode laser absorption spectroscopy, and measurements of all other major stable species were made downstream of...

متن کامل

Kinetic study of low temperature methane oxidation in a nanosecond repetitively pulsed dielectric barrier discharge

Methane oxidation was investigated in a nanosecond repetitively pulsed dielectric barrier discharge. Quantitative measurements of temperature and product species were performed using tunable diode laser absorption spectroscopy and gas chromatograph sampling. Discrepancies with modelling work revealed uncertainties in the low temperature oxidation reactions, particularly for methyl radical oxida...

متن کامل

Electric field measurement in repetitively pulsed nanosecond discharges in a high pressure hydrogen environment

Electric fields of repetitively pulsed nanosecond discharges have been measured from electric-field induced Raman scattering by hydrogen molecules. Especially the temporal evolution of the electric field spatial distribution was recorded. With a high-speed optical emission intensity analysis, it has been found that most ionization events take place within a very short period during an ionizatio...

متن کامل

A ‘frozen electric-field’ approach to simulate repetitively pulsed nanosecond plasma discharges and ignition of hydrogen–air mixtures

High-fidelity modelling of nanosecond repetitively pulsed discharges (NRPDs) is burdened by the multiple time and length scales and large chemistry mechanisms involved, which prohibit detailed analyses and parametric studies. In the present work, we propose a ‘frozen electric-field’ modelling approach to expedite the NRPD simulations without adverse effects on the solution accuracy. First, a bu...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: Journal of Physics D

سال: 2021

ISSN: ['1361-6463', '0022-3727']

DOI: https://doi.org/10.1088/1361-6463/abf61f